Download Localized to Itinerant Electronic Transition in Perovskite by John B. Goodenough PDF
By John B. Goodenough
Content material: common concerns / J.B. Goodenough -- shipping homes / J.B. Goodenough, J.-S. Zhou -- neighborhood atomic constitution of CMR manganites and similar oxides / T. Egami -- Optical spectroscopic stories of metal-insulator transitions in perovskite-related oxides / S.L. Cooper
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Sample text
The volume of such a ¯uctuation would be de®ned by cooperative oxygen displacements of period À12 xÀ1 s; xO is the frequency of the cooperative oxygen displacements O % 10 that de®ne the volume of a second-phase ¯uctuation. Evidence that this is the case comes from photoemission spectroscopy (PES), which is a fast enough experimental probe to see ¯uctuations on time scales shorter than xÀ1 O . Morikawa et al. [11] have performed an elegant study of SrVO3 and CaVO3 with inverse, high-resolution PES (Fig.
A smaller t < 0) favoring the in-phase stacking. The observation [34, 43] that the Curie±Weiss paramagnetic susceptibility has a larger Weiss constant in the temperature interval T > TJT compared with that for TN < T < TJT indicates that the magnetic interactions become isotropically ferromagnetic above TJT. On the assumption that stoichiometric LaMnO3 remains an insulator above TJT, Goodenough et al. [44] postulated a strong electron coupling to dynamic local J-T deformations, which would favor isotropic ferromagnetic superexchange interactions, and the appearance of ferromagnetism in the system LaMn1)xGaxO3 appeared to con®rm that postulate [44, 45].